@article{148291,
  author = {Denise L. Mauzerall and D. Narita and H. Akimoto and L. Horowitz and S. Walters and D. Hauglustaine and B. Brasseur},
  title = {Seasonal Characteristics of Tropospheric Ozone Production and Mixing Ratios Over East Asia: A Global Three-dimensional Chemical Transport Model Analysis},
  abstract = { We examine seasonal and geographical distributions of tropospheric ozone production and mixing ratios over East Asia with a global three-dimensional chemical transport model called Model of Ozone and Related Tracers, version 1 (MOZART-1). Net ozone production within the East Asian boundary layer exhibits three distinct seasonal cycles depending on region (north of 20N, 5-20N and south of 5N). North of 20N, net ozone production over East Asia from spring through autumn is found to have a maximum extending from 25N-40N and from central eastern China to Japan, resulting from the strong emission and transport of anthropogenic O<sub>3</sub>~precursors. In winter, maximum O<sub>3</sub>~production in this region occurs between 20N and 30N. This is a region of long-range transport. Over the Indochina peninsula, between 5N and 20N, net O<sub>3</sub>~production is controlled by the seasonal cycle between wet and dry seasons and has a maximum at the end of the dry season due to emissions from biomass burning. South of 5N, in the true tropics, O<sub>3</sub>~mixing ratios are relatively constant throughout the year and do not exhibit a seasonal cycle. A spring-summer maximum of net O<sub>3</sub>~production is found throughout the troposphere in East Asia. We estimate an annual net O<sub>3</sub>~production in East Asia of 117 Tg/yr. Both model results and analysis of measurements of O<sub>3</sub>-CO correlations over East Asia and Japan show strong variability as a function of both photochemical activity and seasonal meteorology, and indicate ozone export off the coast of East Asia in spring. An upper estimate of O<sub>3</sub>~export from East Asia to the Pacific Ocean in the mid-1980s of 3.3 Gmol/day (58 Tg/yr) is obtained. },
  year = {2000},
  journal = {Journal of Geophysical Research},
  volume = {105},
  pages = {17895-17910},
  language = {eng},
}